Researching ROLL families worldwide: www.rollintl.com/roll/rolldata.htm
Listed below is where I found ROLL families in Switzerland and Alsace. There appears to be a von ROLL coat from Canton Uri and a de ROLLE coat from Canton Genf/Bern or Solothurn.

SWITZERLAND:
NOTE: There were many ROLLE and von ROLL families in Switzerland. “Canton” = State/Province.
Altdorf, Uri, Switzerland***** <1600
Argue valley, Switzerland
Bern Canton, Switzerland [related to Geneva Von ROLLs]
Bernau, Hauptmann, Uri, Switzerland <1667
Biel, Switzerland to USA
Delemont, Switzerland to USA
Fribourg Canton, Switzerland
Fribourg, Fribourg, Switzerland <1680 (from Tarentaise, Loire, Rhône-Alpes, France in 1680 and Cernay, France in 1763)
Fürsprech, Altdorf, Uri, Switzerland <1724
Geneva Canton, Switzerland*** [Von ROLL]
Glarus, Glarus, Switzerland to USA <1685
Hauptmann, Uri, Switzerland <1626
Landammann, Uri, Switzerland <1740
Lausanne, Switzerland to USA
Leuggern, Uri, Switzerland <1648 (Johanniterkumtur zu)
Leutnant, Uri, Switzerland <1668
Matzendorf, Solothurn, Switzerland <1710
Mitlödi,Glarus, Switzerland to USA <1704
Netstal,Glarus, Switzerland to USA <1645
Ritter, Altdorf, Uri, Switzerland <1562
Roggenburg Switzerland to USA
Rolle, Vaud Canton, Switzerland [origination of the Geneva Von ROLLs]***
Soleure Canton, Switzerland [related to Geneva Von ROLL and from Savoie, France]
Soleure, Switzerland to USA
Soleure, Switzerland <1761
Savoie (comete de Savoie), Switzerland (or France?) [ROLLE] <1300 – Jean de ROLLE
Thierachern Switzerland to USA
Uri Canton, Switzerland [Von ROLL, not related to Geneva]
Zurich, Switzerland to USA

FRANCE:
Agde, Hérault Languedoc Roussillon, France to USA
Ambert, Basse-Auvergne, France <1652
Aue, France to USA
Aue, Saxony, France to USA
Bet, France to USA
Biarritz, Pyrenees Atlantiques, Aquitaine France to USA
Biaudos, Landes, Aquitaine, France to USA
Blanc-Mesnil, Seine-St-Denis, France to USA
Bonneville, Haute, Savoie, Rhône Alpes, France to USA
Dordogne, Aquitaine, France to USA
Dürnkrut, Ebenthal, France to USA
Landes Aquitaine France to USA
Leuwarden, France <1781
Marseille, France to USA
Meaux, Seine et Marne, Ile de France, France to USA
Montgé-Dommartin, Seine et Marne, Ile de France, France to USA
Nancy-sur-Cluses, Haute-Savoie, Rhône-Alpes, France <1706
Paris, France to USA
Paris, France <1846
Paris, Paris, Ile de France, France to USA
Roggenburg, France (also Roggenburg, Switzerland?)
Rottenmann, France to USA
Saint Laurent de Gosse (Château de Montpellier) Landes Aquitaine, France to USA
Savoie, a second-order administrative division, France
Sevran, Seine St. Denis, Ile de France, France to USA
St. Nicolas or Anthelupt, France <1872
Tarentaise, Loire, Rhône-Alpes, France <1680
Val d'Oise, Ile de France, France to USA
Vienne, Poitiers, France <1790
Vosges. a second-order administrative division, France (150 miles NW of Basel, Switzerland)
Wolfersdorf, France >1684

Alsace-Lorraine (Elsass/Elsaß/Alsatia), FRANCE (was part of Germany between 1870-1919)
Aspach-le-Haut, Haut-Rhin, Alsace, France (from Steinzoultz, France)
Aspach-le-Haut, Haut-Rhin, Alsace, France <1770
Barr, Bas Rhin, Alsace, France to USA
Bayonne, Pyrénées Atlantiques, Aquitaine, France to USA
Bellemagny, France >1650
Bellemagny, Haut Rhin, Alsace, France to USA
Bettlach, Haut Rhin, Alsace, France to USA
Bourg/Raedersdorf, Haut-Rhin, Alsace, France <1713
Bouxwiller, Bas-Rhin, Alsace, France <1826
Carspach, Haut Rhin, Alsace, France to USA
Cernay, Haut-Rhin, Alsace, France <1635 (probably related to Savoie, France ROLLs)
Dannemarie, Haut Rhin, Alsace, France to USA
Dannermarie, France <1700
Delle, Territoire de Belfort, Franche Comté France to USA
Delle, Territorie de Belfort, Franche Comté, France <1788
Dettwiller, Bas Rhin, Alsace, France to USA
Dettwiller, Bas-Rhin, Alsace, France (aka Alsace, Germany)***** <1770
Dornach, near Mulhouse, Haut-Rhin, Alsace, France <1722 (from Bourg, France)
Eschentzwiller, Haut-Rhine, Alsace, France <1587
Folgensbourg, Haut-Rhin, Alsace, France >1759
Grandvillars, Terr. de Belfort, Franche Comté, France to USA
Guebwiller, Haut-Rhin, Alsace, France - early 1600’s
Guewenheim, Haut Rhin, Alsace, France to USA
Guewenheim, Haut-Rhin, Alsace, France <1648
hau, Hochstatt, Haut Rhin, Alsace, France to USA
Hayange, Moselle, Lorraine, France <1708
Hayange, Moselle, Lorraine, France to USA
Hochstatt, Haut-Rhin, Alsace, France >1710 (from Bourg, France)
Kiffis, Haut Rhin, Alsace France to USA
Kiffis, Haut Rhin, Alsace, Germany (now France))***** <1700
Kirchberg, Haut-Rhin, Alsace France to USA
Landser, Haut-Rhin, Alsace, France >1706 (from Nancy-sur-Cluses, Haute-Savoie, Rhône-Alpes, France)
Leimbach, Haut-Rhin, Alsace, France <1615
Marschpich, Lorraine, France to USA
Masevaux, Haut-Rhin, Alsace, France (from Canton Soleure, Switzerland)
Monsvillers, France to USA
Monswiller, Bas Rhin Alsace, France to USA
Monswiller, Bas-Rhin, Alsace, France***** <1706
Moselle, Lorraine, France to USA
Muespach-le-Bas, Haut-Rhin, Alsace, France <16981753 (from Bourg, France in 1710)
Mulheuse, France to USA
Mulhouse, Haut Rhin, Alsace, France to USA
Mulhouse, Haut Rhin, Alsace, Germany (now France) <1842
Mulhouse, Haut-Rhin, Alsace, France (from Uffholtz, France)
Niederschaeffolsheim, Bas Rhin, France to USA
Oberbruck, Haut-Rhin, Alsace, France to USA
Ottersthal, Bas Rhin, Alsace, France to USA
Reichshoffen, Bas Rhin France to USA
Saessolsheim, Bas Rhin, Alsace France to USA
Saverne, Bas Rhin Alsace, France to USA
Scionzier, Haute Savoie Rhône Alpes, France to USA
Seppois-le-Bas, Haut-Rhin, Alsace, France [Pierre Louis de ROLL, related to Canton Uri]
Sewen, Haut Rhin, Alsace, France to USA
Sewen, Haut-Rhin, Alsace, France >1710 (from Matzendorf, Solothurn, Switzerland)
Steinsoultz, Haut-Rhin, Alsace, France
Strasbourg or Bouxwiller (Erstein?), Alsace, France <1770
Thann, Haut-Rhin, Alsace, France <1629 (related to Cernay, France ROLLs)
Uffholtz, Haut-Rhin, Alsace, France <1573 (related to Mulhouse, France ROLLs)
Vieux-Ferrette, Haut Rhin, France Haut Rhin Alsace France to USA
Waldighofen, Haut-Rhin, Alsace, France <1696
Waldolwisheim, Bas Rhin, Alsace France to USA
Wegscheid (Wegsheid), Haut Rhin, Alsace France to USA
Wegscheid, Haut-Rhin, Alsace, France*** <1766
Weyersheim, Brumath, Bas-Rhin, France [ROLLI/ROLI] <1733
Wingersheim, Bas Rhin, Alsace France to USA
Zillisheim, Haut Rhin, Alsace France to USA